研究团队

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原烨,硕士生导师

基本情况

出生年月:1988-12        籍贯:山西
学历:武汉理工大学,材料科学与工程博士;材料科学与工程、应用化学双学士
工作单位:武汉理工大学材料复合新技术国家重点实验室
联系地址:武汉市洪山区武汉理工大学南湖校区化学楼1楼特1室
联系电话:+86-18635800380 QQ:616181394
Email:fyyuanye@whut.edu.cn

研究领域

1. 二氧化碳的捕获与转化利用(CCU);
2. 绿色化学,高价值精细化学品合成;
3. 有机金属催化剂和多孔催化材料的制备与应用;

教育经历

2012/06–2017/10:武汉理工大学,材料科学与工程,工学博士,
导师:Francis Verpoort教授
2008/09–2012/06:武汉理工大学,材料科学与工程, 工学学士,
武汉理工大学,应用化学,理学学士

科研项目

1. 国家自然科学基金青年项目(项目批准号:22102127),基于金属簇合物催化的双取代碳酸亚乙烯酯的新合成路线研究,2022-01至2024.12,24万,在研,主持
2. 齐鲁工业大学(山东省科学院)生物基材料与绿色造纸国家重点实验室开放基金, (项目批准号:GZKF202023), 生物质基离子液体在CO2催化转化中的应用, 2021-01至2022-12, 6万, 在研, 主持
3. 国家自然科学基金委外国青年学者研究基金延续项目(项目批准号:21950410754),金属在MOFs 衍生的功能化碳基体的分散及其前驱体作为一种强而有效的催化剂用于CO2转化,绿色化学和能源,2020/01-2021/12,30万,在研,参与
4. 国家自然科学基金外国青年学者研究基金项目(项目批准号:21850410449),MOFs衍生的分散在碳基体中的金属作为有效的二氧化碳转化催化剂,2019/01-2019/12,20万,参与,已结题
5. 青年科学基金项目 (项目批准号:21502146),金属有机骨架材料开发及绿色能源净化与绿色化学催化应用,2016/01-2018/12,21万,参与,已结题

工作经历

2017/11至今:武汉理工大学,材料复合新技术国家重点实验室

代表性论文与专利(*通讯作者)

(1) CO2-Induced Dissolution of ZnO into Ionic Liquids and Its Catalytic Application for the Hydration of Propargylic Alcohols. Yongxing Zhang, Jia Hu, Yong Xu, Xiangyu Yan, Siqi Zhang, Kang Duan, Cheng Chen, Ye Yuan, Francis Verpoort. Applied Catalysis B: Environmental, 2022, 310, 121270.
(2) A Green and Recyclable CuSO4·5H2O/Ionic Liquid Catalytic System for the CO2-Promoted Hydration of Propargyl Alcohols: An Efficient Assembly of α-Hydroxy Ketones. Ye Yuan; Jia Hu; Yu Wang; Leilei Huang; Jiayun Zheng; Yufeng Zhao; Yiyun Chen; Cheng Chen; Francis Verpoort. J. Cat, 2022, 405, 561-570.
(3) Du, M.; Gong, Y.; Bu, C.; Hu, J.; Zhang, Y.; Chen, C.; Chaemchuen, S.; Yuan, Y.; Verpoort, F., An efficient and recyclable AgNO3/ionic liquid system catalyzed atmospheric CO2 utilization: Simultaneous synthesis of 2-oxazolidinones and α-hydroxyl ketones. Journal of Catalysis 2021, 393, 70-82.
(4) Chen, C.; Wang, Z.-Q.; Gong, Y.-Y.; Wang, J.-C.; Yuan, Y.; Cheng, H.; Sang, W.; Chaemchuen, S.; Verpoort, F., Cobalt embedded in nitrogen-doped porous carbon as a robust heterogeneous catalyst for the atom-economic alcohol dehydrogenation to carboxylic acids. Carbon 2021, 174, 284-294.
(5) Tandem Reactions Based on the Cyclization of Carbon Dioxide and Propargylic Alcohols: Derivative Applications of α-Alkylidene Carbonates, Bowen Jiang, Xiangyu Yan, Yong Xu, Natalya Likhanova, Heriberto Díaz Velázquez, Yanyan Gong, Ye Yuan 1, and Francis Verpoort, Catalysts, 2022, 12, 73.
(6) Zeolitic imidazolium frameworks-derived Ru-based composite materials enable the catalytic dehydrogenation of alcohols to carboxylic acids. Zhan Chen, Jing Hang, Song Zhang, Ye Yuan *, Francis Verpoort *, Cheng Chen, Catalysts, accepted 2023.
(7) Green Synthesis of 2-Oxazolidinones by an Efficient and Recyclable CuBr/Ionic Liquid System viaCO2, Propargylic alcohols, and 2-Aminoethanols. Chao Bu, Yanyan Gong, Minchen Du, Cheng Chen, Somboon Chaemchuen, Jia Hu, Yongxing Zhang, Heriberto Díaz Velázquez, Ye Yuan, Francis Verpoort. Catalysts, 2021, 11(2), 233.
(8) Minchen Du; Yanyan Gong; Chao Bu; Jia Hu; Yongxing Zhang; Cheng Chen; Somboon Chaemchuen; Ye Yuan*; Francis Verpoort*; An efficient and recyclable AgNO3/ionic liquid system catalyzed atmospheric CO2 utilization: Simultaneous synthesis of 2-oxazolidinones and α-hydroxyl ketones, Journal of Catalysis, 2021, 393: 70-82. (IF:7.92)
(9) Chao Bu, Yanyan Gong, Minchen Du, Cheng Chen, Somboon Chaemchuen, Jia Hu, Yongxing Zhang, Heriberto Díaz Velázquez, Ye Yuan*, and Francis Verpoort*, Green Synthesis of 2-Oxazolidinones by an Efficient and Recyclable CuBr/Ionic Liquid System via CO2, PropargylicAlcohols, and 2-Aminoethanols, Catalysts, 2021, 11: 233(IF:4.146)
(10) Di Li; Yanyan Gong; Minchen Du; Chao Bu; Cheng Chen; Somboon Chaemcheun; Jia Hu; Yongxing Zhang; Ye Yuan*; Francis Verpoort*; CO2 Promoted Hydration of Propargylic Alcohols: Green Synthesis of α Hydroxy Ketones by an Efficient and Recyclable AgOAc/Ionic Liquid System, ACS Sustainable Chemistry & Engineering, 2020, 8: 8148-8155. (IF:8.198)
(11) Somboon Chaemchuen; Xuan Xiao; Marzieh Ghadamyari; Bibimaryam Mousavi; Nikom Klomkliang; Ye Yuan*; Francis Verpoort*; Robust and efficient catalyst derived from bimetallic Zn/Co zeolitic imidazolate frameworks for CO2 conversion, Journal of Catalysis, 2019, 370: 38-45. (IF:7.92)
(12) Li Di,Du Min-chen,Bu Chao,Chen Cheng,Hu Jia,Zhang Yong-xing,Yuan Ye*,Francis Verpoort*,Three-component Reactions of Propargyl Alcohols,Secondary Amines and CO2 Catalyzed by CuCl2/IonicLiquids, Journal of Molecular Catalysis (China), 2019,33, 543
(13) Dandan Song; Di Li; Xuan Xiao; Chen Cheng; Somboon Chaemchuen; Ye Yuan*; Francis Verpoort*; Synthesis of β-oxopropylcarbamates in a recyclable AgBr/ionic liquid catalytic system: An efficient assembly of CO2 under ambient pressure, Journal of CO2 Utilization, 2018, 27, 217-222. (IF:7.132)
(14) Cheng Chen, Yang Miao, Kimmy De Winter, Hua-Jing Wang, Patrick Demeyere, Ye Yuan,* and Francis Verpoort,* Ruthenium-Based Catalytic Systems Incorporating a Labile Cyclooctadiene Ligand with N-Heterocyclic Carbene Precursors for the Atom-Economic Alcohol Amidation Using Amines, Molecules 2018, 23, 2413(IF:4.411)
(15) Ye Yuan; Yu Xie; Cheng Zeng; Dandan Song; Somboon Chaemchuen; Cheng Chen*; Francis Verpoort*; A recyclable AgI/OAc− catalytic system for the efficient synthesis of α-alkylidene cyclic carbonates: carbon dioxide conversion at atmospheric pressure, Green Chemistry, 2017, 19, 2936-2940. (IF:10.182)
(16) Ye Yuan, Cheng Chen, Cheng Zeng, Bibimaryam Mousavi, Somboon Chaemchuen, and Francis Verpoort*, Carboxylation of Terminal Alkynes with Carbon Dioxide Catalyzed by an In Situ Ag2O/N-Heterocyclic Carbene Precursor System, ChemCatChem 2017, 9, 882-887. (IF:5.686)
(17) Ye Yuan, Yu Xie, Cheng Zeng, Dandan Song, Somboon Chaemchuen, Cheng Chen* and Francis Verpoort*, A simple and robust AgI/KOAc catalytic system for the carboxylative assembly of propargyl alcohols and carbon dioxide at atmospheric pressure, Catal.Sci.Technol., 2017, 7, 2935–2939(IF:6.119)
(18) Ye Yuan, Yu Xie, Dandan Song, Cheng Zeng, Somboon Chaemchuen, Cheng Chen, Francis Verpoort*, One-pot carboxylative cyclization of propargylic alcohols and CO2 catalysed by N-heterocyclic carbene/Ag systems, Appl Organometl Chem. 2017; e3867(IF:4.105)
(19) Yanyan Gong, Ye Yuan, Cheng Chen, Somboon Chaemchuen*, Francis Verpoort*, Palladium metallated shell layer of shell@core MOFs as an example of an efficient catalyst design strategy for effective olefin hydrogenation reaction, Journal of Catalysis, 2020, 392, 141-149.
(20) Yanyan Gong, Ye Yuan, Cheng Chen, Pan Zhang, Jichao Wang, Serge Zhuiykov, Somboon Chaemchuen, Francis Verpoort, Core-shell metal-organic frameworks and metal functionalization to access highest efficiency in catalytic carboxylation, Journal of Catalysis, 2019, 371, 106-115.
(21) CO2-Promoted Hydration of Propargylic Alcohols: Green Synthesis of α-Hydroxy Ketones by an Efficient and Recyclable AgOAc/Ionic Liquid System. Li, Di ; Gong, Yanyan; Du, Minchen; Bu, Chao; Chen, Cheng; Chaemchuen, Somboon; Hu, Jia; Zhang, Yongxing; Yuan, Ye; Verpoort, Francis, ACS Sustainable Chem. Eng. 2020, https://doi.org/10.1021/acssuschemeng.9b07546
(22) Yanyan Gong, Ye Yuan, Cheng Chen, Pan Zhang, Jichao Wang, Somboon Chaemchuen, Francis Verpoort, Enhancing catalytic performance via structure core-shell metal-organic frameworks, Journal of Catalysis, 2019, 375, 371-379.
(23) Cheng Chen, Zhi-Qin Wang, Yan-Yan Gong, Ji-Chao Wang, Ye Yuan, Hua Cheng, Wei Sang, Somboon Chaemchuen*, Francis Verpoort*. Cobalt embedded in nitrogen-doped porous carbon as a robust heterogeneous catalyst for the atom-economic alcohol dehydrogenation to carboxylic acids, Carbon, 2021, 174, 284-294.
(24) Zhi-Qin Wang; Xiao-Sheng Tang; Zhao-Qi Yang; Bao-Yi Yu, Hua-Jing Wang; Wei Sang, Ye Yuan, Cheng Chen*; Francis Verpoort*; Highly active bidentate N-heterocyclic carbene/ruthenium complexes performing dehydrogenative coupling of alcohols and hydroxides in open air, Chem. Commun. 2019, 55, 8591-8594.
(25) Xuan-Jun Wu, Hua-Jing Wang, Zhao-Qi Yang, Xiao-Sheng Tang, Ye Yuan, Wei Su, Cheng Chen* and Francis Verpoort*, Efficient and phosphine-free bidentate N-heterocyclic carbene/ruthenium catalytic systems for the dehydrogenative amidation of alcohols and amines, Org. Chem. Front. 2019, 6, 563-570.
(26) Wei Sang, Yan-Yan Gong, Hua Cheng, Rui Zhang, Ye Yuan, Guang-Gao Fan, Zhi-Qin Wang, Cheng Chen*, Francis Verpoort*, Transition-Metal-Free Base-Controlled C-N Coupling Reactions: Selective Mono Versus Diarylation of Primary Amines with 2-Chlorobenzimidazoles, Adv. Synth. Catal., 2021, 363, 1408-1416.
(27) Wei Sang, Ayao Jean Gavi, Bao-Yi Yu, Hua Cheng, Ye Yuan, Yuan Wu, Petra Lemmens, Cheng Chen*; Francis Verpoort*. Palladium-Catalyzed Ligand-Free C-N Coupling Reactions: Selective Diheteroarylation of Amines with 2-Halobenzimidazoles, Chem. - Asian J., 2020, 15, 129-135.
(28) Wan-Qiang Wang, Hua Cheng, Ye Yuan, Yu-Qing He, Hua-Jing Wang, Zhi-Qin Wang, Wei Sang, Cheng Chen*, Francis Verpoort*. Highly Efficient N-Heterocyclic Carbene/Ruthenium Catalytic Systems for the Acceptorless Dehydrogenation of Alcohols to Carboxylic Acids: Effects of Ancillary and Additional Ligands, Catalysts, 2020, 10, 10.
(29) Hua Cheng, Maoqian Xiong, Ni Zhang, Huajing Wang, Yang Miao, Wei Su, Ye Yuan, Cheng Chen*, Francis Verpoort*. Efficient N-heterocyclic carbene/ruthenium catalytic systems for the alcohol amidation with amines: Involvement of poly-carbene complexes? ChemCatChem, 2018, 10, 4338-4345.
(30) Wan-Qiang Wang, Ye Yuan, Yang Miao, Bao-Yi Yu, Hua-Jing Wang, Zhi-Qin Wang, Wei Sang, Cheng Chen*, Francis Verpoort*. Well-defined N-heterocyclic carbene/ruthenium complexes for the alcohol amidation with amines: The dual role of cesium carbonate and improved activities applying an added ligand, Appl. Organomet. Chem. 2020, 34, e5323.
(31) Haotian Wu, Rongrong Hou, Ye Yuan, Jingli Zhang,* Bifeng Chen, Taolei Sun*, Highly Regioselective Synthesis of 1-Acyl-5-hydroxypyrazolines or Synthesis of 3,5-Disubstituted Pyrazoles from (E)-β-Chlorovinyl Ketones and Benzohydrazides or Hydrazine Hydrate, HETEROCYCLES, 2020, 100, 916-933.
(32) Guangyong Shi, Wei Xu, Jichao Wang, Ye Yuan, Somboon Chaemchuen*, Francis Verpoort*, A Cu-based MOF for the effective carboxylation of terminal alkynes with CO2 under mild conditions, Journal of CO2 Utilization, 2020, 39, 101177.
(33) Youchi Zhang, Jingli Zhang*, Ye Yuan, Liran Liu, Bifeng Chen, Taolei Sun*, Synthesis of Polysubstituted 2H-Pyran-2-ones or Phenols via One-Pot Reaction of (E)-β-Chlorovinyl Ketones and Electron-Withdrawing Group Substituted Acetates or β-Diketones, European Journal of Organic Chemistry, 2020, 13 1976-1986.
(34) Xing Yang, Ze-Hun Cao, Yang Zhou, Feng Cheng, Zi-Wei Lin, Zhi Ou, Ye Yuan, Yi-Yong Huang*, Petasis-Type gem-Difluoroallylation Reactions Assisted by the Neighboring Hydroxyl Group in Amines, Organic Letters, 2018, 20, 2585-2589.
(35) Bibimaryam Mousavi, Somboon Chaemchuen, Chizoba I. Ezugwu, Ye Yuan, Francis Verpoort*, The effect of synthesis procedure on the catalytic performance of isostructural ZIF-8, Applied Organometallic Chemistry, 2018, 32, e4062.