研究团队

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Somboon Chaemchuen,副研究员、硕士生导师

基本情况

出生年月:1984-09        籍贯:泰国
最高学历:泰国朱拉隆功大学 ,化学工程博士
工作单位:武汉理工大学 材料复合新技术国家重点实验室
联系地址:武汉市洪山区武汉理工大学南湖校区化学楼1楼312室
联系电话:13871122862
Email:sama_che@hotmail.com

研究领域

金属有机骨架(MOFs)或其衍生材料的结构设计、制备及在气体吸附/分离与(电)催化方面的应用,具体包括:
1. 利用这些材料的可设计性与功能化来提升其性能;
2. 研究绿色新材料的合成方法并明确其结晶机理;
3. 将所得材料用于 CO2 吸附、沼气分离、CO2 转化、生物聚合或电催化等领域;

教育经历

2007/04–2011/06:泰国朱拉隆功大学,催化和催化反应工程实验室,工程学院,化学工程博士
2003/05–2007/04:泰国玛希隆大学 ,工程学院,化学工程专业,工学学士

科研项目

1. 国家自然科学基金委外国青年学者研究基金延续项目(项目批准号:21950410754),金属在MOFs 衍生的功能化碳基体的分散及其前驱体作为一种强而有效的催化剂用于CO2转化,绿色化学和能源,2020/01-2021/12,30万,项目负责人,在研
2. 国家自然科学基金外国青年学者研究基金项目(项目批准号:21850410449),MOFs衍生的分散在碳基体中的金属作为有效的二氧化碳转化催化剂,2019/01-2019/12,20万,项目负责人,已结题
3. 青年科学基金项目 (项目批准号:21502146),金属有机骨架材料开发及绿色能源净化与绿色化学催化应用,2016/01-2018/12,21万,项目负责人,已结题
4. 武汉理工大学新教师研究基金(项目批准号:163143003),金属有机骨架材料在清洁能源中的应用,2015/01-2017/01,5万,项目负责人,已结题
5. 博士后研究基金,金属-有机骨架的合成与应用,2012/01-2014/01,2万,项目负责人,已结题
6. 国家研究型大学计划,用甲烷进行CO2重整催化剂的开发,2011/01-2014/01,2万,项目负责人,已结题
7. 皇家金禧年博士项目,应用于乙烯和2-丁烯歧化反应的钨支撑材料,2007/01-2010/01,4万,项目负责人,已结题

工作经历

2016/11-至今:武汉理工大学材料复合新技术国家重点实验室,副研究员
2015/03-2016.10:武汉理工大学材料复合新技术国家重点实验室,助理研究员
2012/06-2014.12:武汉理工大学材料复合新技术国家重点实验室,博士后

代表性论文与专利(*通讯作者)

(1) Z. Wang, X. Hou, S. Dekyvere, B. Mousavi and S. Chaemchuen, Single-thermal synthesis of bimetallic Co/Zn@NC under solvent-free conditions as an efficient dual-functional oxygen electrocatalyst in Zn–air batteries, Nanoscale, 2022, 14, 16683-16694.
(2) N-functionalized hierarchical carbon composite derived from ZIF-67 and carbon foam for efficient overall water splitting. Jichao Wang, Somboon Chaemchuen, Cheng Chen, Philippe M. Heynderickx, Soumyajit Roy and Francis Verpoort, Journal of Industrial and Engineering Chemistry, 105, 2022, 222-230.
(3) Q. Wu, J. Gu, J. Wang, N. Liu and S. Chaemchuen, Impact in rational synthesis Co-ZIF templates for derived the structural Co@NC catalysis for high efficient hydrogen and oxygen evolution reactions, International Journal of Hydrogen Energy, 2023, 48, 2663-2676.
(4) Chen, C.; Wang, Z.-Q.; Gong, Y.-Y.; Wang, J.-C.; Yuan, Y.; Cheng, H.; Sang, W.; Chaemchuen, S.; Verpoort, F., Cobalt embedded in nitrogen-doped porous carbon as a robust heterogeneous catalyst for the atom-economic alcohol dehydrogenation to carboxylic acids. Carbon 2021, 174, 284-294.
(5) Chaemchuen, S.; Dai, Q.; Wang, J.; Zhu, C.; Klomkliang, N.; Yuan, Y.; Cheng, C.; Elkadi, M.; Luo, Z.; Verpoort, F., Enhancing catalytic activity via metal tuning of zeolitic imidazole frameworks for ring opening polymerization of l-lactide. Applied Catalysis A: General 2021, 624, 118319.
(6) Bimetallic-doped Zeolitic imidazole framework-derived Cobalt-Nitrogen-Carbon supported on reduced graphene oxide enabling Efficient Microwave Absorption. Qi Chen, Xiaogang Su, Xing Liu, Jichao Wang, Rongguo Song, Daping He, Somboon Chaemchuen, and Francis Verpoort, J Taiwan Inst Chem Eng, Volume, 2022, 134, 104350.
(7) In-situ thermal solvent-free synthesis of zeolitic imidazolate frameworks with high crystallinity and porosity for effective adsorption and catalytic applications. Jichao Wang, Somboon Chaemchuen, Nikom Klomkliang, Francis Verpoort, Cryst. Growth Des. 2021, 21, 9, 5349–5359.
(8) Z. Zheng, J. Wang, M. Liu, B. Mousavi, N. Liu and S. Chaemchuen, Facile and green synthesis cobalt embedded in N-doped porous carbon under zeo-waste conditions as an efficient oxygen evolution reduction catalyst, Microporous and Mesoporous Materials, 2022, 337, 111916.
(9) X. Hou, J. Wang, B. Mousavi, N. Klomkliang and S. Chaemchuen, Strategies for induced defects in metal–organic frameworks for enhancing adsorption and catalytic performance, Dalton Transactions, 2022, 51, 8133-8159.
(10) Carbon-Supported Cobalt Nanoparticles via Thermal Sugar Decomposition as Efficient Electrocatalysts for the Oxygen Evolution Reaction. Wang, Jichao, Liu, Meng, Chaemchuen Somboon, Klomkliang, Nikom, Kao Chih-Ming, Verpoort Francis. ACS Applied Nano Materials, 2022, 5, 7993-8004.
(11) Metal Embedded Porous Carbon for Efficient CO2 Cycloaddition under Mild Conditions, Chen Qi, Somboon Chaemchuen, Meng Liu, Jichao Wang, Serge Zhuiykov and Francis Verpoort. Catalysts 2022, 12(4), 427.
(12) Somboon Chaemchuen, Zhonghan Cheng, Xiaotong Hou, Francis Verpoort, Jakkapan Kumsi, Nikom Klomkliang, Solid–solid thermal synthesis of bimetallic Ni/Zn embedded in N-doped porous carbon for efficient adsorptive separation based on CO2 adsorption at low pressure, Fuel, Volume 356, 2024, 129608, ISSN 0016-2361, https://doi.org/10.1016/j.fuel.2023.129608.
(13) Zeolitic Imidazolate Framework-8 as an Efficient and Facile Heterogeneous Catalyst for the Acceptorless Alcohol Dehydrogenation to Carboxylates. Jun-Fei Gu, Cheng Chen, Zhong-Hui Zheng, Jing Hang, Wei Sang, Ji-Chao Wang, Ye Yuan, Somboon Chaemchuen, and Francis Verpoort. J. Cat. 2023, 417, 202-212.
(14) Z. Li, S. Chaemchuen, Chem. Rec. 2023, 23, e202300142.
(15) Solvent-free synthesis of Co/CoNx encapsulated by N-doped, sucrose-derived porous carbon as bifunctional air cathode catalyst for high-energy rechargeable zinc-air batteries, Sander Dekyvere, Somboon Chaemchuen, Zhonghui Zheng, Jichao Wang, Meng Liu, Francis Verpoort*, Journal of Alloys and Compounds, 2023, accepted.
(16) Thermal Solid–Solid Transformation Synthesis of Zinc Anchored in Hierarchical Porous N-Doped Carbon for Efficient CO2 Applications. Somboon Chaemchuen; Xiaotong Hou; Zhonghan Cheng; Kui Zhou; Serge Zhuiykov; Francis Verpoort. Energy & Fuels, DOI: 10.1021/acs.energyfuels.2c03949.
(17) Rational Design of Cobalt Catalysts Embedded in N-Doped Carbon for the Alcohol Dehydrogenation to Carboxylic Acids. Cheng Chen, Jing Hang, Zhi-Qin Wang, Zhong-Hui Zheng, Jun-Fei Gu, Wei Sang, Ye Yuan, Somboon Chaemchuen, Francis Verpoort. Molecular Catalysis, 2023, 535, 112891.
(18) Chen C., Wang Z.Q., Gong Y.Y., Wang J., Yuan Y., Cheng H., Sang W., Chaemchuen S.*, Verpoort F.*, Cobalt embedded in nitrogen-doped porous carbon as a robust heterogeneous catalyst for the atom-economic alcohol dehydrogenation to carboxylic acids, Carbon, 2020, 174, 284-294, DOI: 10.1016/j.carbon.2020.12.040.
(19) Gong Y, Yuan Y, Chen C, Chaemchuen S.*, Verpoort F.*, Palladium metallated shell layer of shell@ core MOFs as an example of an efficient catalyst design strategy for effective olefin hydrogenation reaction. Journal of Catalysis. 2020, 392,141-149.
(20) Shi G., Xu W., Wang J., Yuan Y., Chaemchuen S.*, Verpoort F.* A Cu-based MOF for the effective carboxylation of terminal alkynes with CO2 under mild conditions. Journal of CO2 Utilization, 2020, 39, 101177
(21) Akimana E., Wang J., Likhanova N.V., Chaemchuen S.*, Verpoort F.*, MIL-101(Cr) for CO2 Conversion into Cyclic Carbonates, Under Solvent and Co-Catalyst Free Mild Reaction Conditions, Catalysts, 2020, 10, 453; doi:10.3390/catal10040453
(22) Chaemchuen S, Heynderickx PM*, Verpoort F.*, Kinetic modeling of oleic acid esterification with UiO-66: from intrinsic experimental data to kinetics via elementary reaction steps. Chemical Engineering Journal, 2020, 394, 124816, DOI: 10.1016/j.cej.2020.124816
(23) Xu, W., Wang, J., Zhang, P., Klomkliang, N., Chaemchuen, S.*, Verpoort, F.* Hierarchical ZIFs@Al2O3 composite materials as effective heterogeneous catalysts, Microporous and Mesoporous Materials, 2020, 297, 110009, DOI: 10.1016/j.micromeso.2020.110009
(24) Shi, G., Xu, W., Wang, J., Mousavi, B., Klomkliang, N., Chaemchuen S.*, Thermochemical transformation in single-step synthesis zeolitic imidazole frameworks under solvent-free. Dalton Transactions, 2020, DOI: 10.1039/C9DT04505H.
(25) Chaemchuen, S., Semyonov, O. V., Dingemans, J., Xu, W., Zhuiykov, S., Khan, A., & Verpoort, F. (2019). Progress on Catalyst Development for Direct Synthesis of Dimethyl Carbonate from CO2 and Methanol. Chemistry Africa, 2019, 2(4), 533-549.
(26) Gong, Y., Yuan, Y., Chen, C., Zhang, P., Wang, J., Khan, A., Zhuikov S., Chaemchuen S.*, Verpoort, F.*, Enhancing catalytic performance via structure core-shell metal-organic frameworks. Journal of Catalysis, 2019, 375, 371-379.
(27) Naz, F., Mumtaz, F., Chaemchuen, S.* and Verpoort, F.*, Bulk Ring-Opening Polymerization of ε-Caprolactone by Zeolitic Imidazolate Framework. Catalysis Letters, 2019, 1-10.
(11) Naz F., Mousavi B., Luo Z., Jabbour C., Heynderickx P. M., Chaemchuen S.*, Verpoort F.*, Switching from linear to cyclic δ-Polyvalerolactone synthesized via Zeolitic Imidazolate Framework as catalyst: A promising approach., Applied Organometallic Chemistry, Accepted 2019.
(28) Patent: PCT/CN2016/085221, WO/2017/210874, IMPERFECT MOFS (IMOFS) MATERIAL, PREPARATION AND USE IN CATALYSIS, SORPTION AND SEPARATION, Inventors: VERPOORT, Francis Walter Cornelius; CHAEMCHUEN, Somboon, 2019.
(29) Gong, Y., Yuan, Y., Chen, C., Zhang, P., Wang, J., Chaemchuen, S*, Verpoort F., Core-shell metal-organic frameworks and metal functionalization to access highest efficiency in catalytic carboxylation, Journal of Catalysis, 2019, 371, 106-115.
(30) Chaemchuen, S., Xiao, X., Ghadamyari, M., Mousavi, B., Klomkliang, N., Yuan, Y., & Verpoort, F., Robust and efficient catalyst derived from bimetallic Zn/Co zeolitic imidazolate frameworks for CO2 conversion, Journal of Catalysis, 2019, 370, 38-45.
(31) Chaemchuen, S., Zhou, K., Yusubov, M.S., Postnikov, P.S., Klomkliang N., Verpoort F., Solid-state transformation in porous metal-organic frameworks based on polymorphic-pillared net structure: Generation of tubular shaped MOFs, Microporous and Mesoporous Materials, 2019, 278:99-104.
(32) Chaemchuen, S., Wang, J. C., Gilani, A. G., & Francis, F. V. Metal-organic frameworks applied for water purification, Resource-Efficient Technologies, 2018, 1: 1-16.
(33) Chaemchuen, S., Xiao, X., Klomkliang, N., Yusubov, M., & Verpoort, F., Tunable Metal–Organic Frameworks for Heat Transformation Applications, Nanomaterials, 2018, 8(9): 661.
(34) Chaemchuen, S., Zhou, K., Mousavi, B., Ghadamyari, M., Heynderickx, P.H., Zhuiykov, S., Yusubov, M.S., & Verpoort, F., Spray drying of zeolitic imidazolate frameworks: investigation of crystal formation and properties, CrystEngComm, 2018, 20(25): 3601-3608.
(19) Zhou, K., Chaemchuen, S.*, Metal-Organic Framework as Catalyst in Esterification of Oleic Acid for Biodiesel Production, International Journal of Environmental Science and Development, 2017, 8(4): 251 DOI: 10.18178/ijesd.2017.8.4.957.
(35) Chaemchuen S, Zhou K, Verpoort F. From biogas to biofuel: materials used for biogas cleaning to biomethane, ChemBioEng Reviews, 2016, 3(6): 250-265.
(36) Chaemchuen, S., Luo, Z., Zhou, K., Mousavi, B., Phatanasri, S., Jaroniec, M., & Verpoort, F., Defect formation in metal–organic frameworks initiated by the crystal growth-rate and effect on catalytic performance, Journal of Catalysis, 2017, 354: 84-91.
(37) Suriye, K., Jareewatchara, W., Lekngarm, P., Chaemchuen, S., Sutthiumporn, K., & Nonkhamwong, A., Metathesis catalyst on mixed metal oxide-zeolite support and process for use thereof, U.S. Patent Application No. 15/515,732. Patent No. WO2016068814A1, PCT/TH2014/000051, 2017.
(38) Zhou, K., Mousavi, B., Luo, Z., Phatanasri, S., Chaemchuen, S.*, & Verpoort, F, Characterization and properties of Zn/Co zeolitic imidazolate frameworks vs. ZIF-8 and ZIF-67, Journal of Materials Chemistry A, 2017, 5(3): 952-957.
(39) Chaemchuem, S., Kui, Z., & Verpoort, F., Control of interpenetration via in situ lithium incorporation in MOFs and their gas adsorption properties and selectivity, CrystEngComm, 2016, 18(39): 7614-7619.
(40) Chaemchuen, S., Zhou, K., Kabir, N. A., Chen, Y., Ke, X., Van Tendeloo, G., & Verpoort, F., Tuning metal sites of DABCO MOF for gas purification at ambient conditions, Microporous and Mesoporous Materials, 2015, 201: 277-285.
(41) Chaemchuen, S., Zhou, K., Yao, C., Luo, Z., & Verpoort, F., Alkali-Metal Tuning of Adsorption Sites in Metal Organic Frameworks MOF-5 for Carbon Dioxide/Methane Separation at Ambient Conditions, Chinese Journal of Applied Chemistry, 2015, 32(5): 552-556.
(42) Chaemchuen, S., Kui, Z. H. O. U., Chen, Y. A. O., Zhi-Xiong, L., & Verpoort, F., Lithium Incorporating Simultaneous with MOF-5 Synthesis for CO2/CH4 Mixed-Gas Separation, CHINESE JOURNAL OF INORGANIC CHEMISTRY, 2015, 31(3): 509-513.
(43) Chaemchuen, S., Kabir, N. A., Zhou, K., & Verpoort, F. Metal–organic frameworks for upgrading biogas via CO2 adsorption to biogas green energy, Chemical Society Review, 2013, 42(24): 9304-9332.